石墨烯基吸波复合材料研究进展

doi:10.11901/1005.3093.2023.114

材料研究学报

2024, Vol. 38

Issue (1): 1-13 DOI: 10.11901/1005.3093.2023.114

综述

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石墨烯基吸波复合材料研究进展

徐东卫¹^,², 王瑞琪¹, 陈平¹(

)

1 大连理工大学化工学院精细化工国家重点实验室大连 116024
2 郑州航空工业管理学院材料学院郑州 450046

Research Progress of Graphene-based Absorbing Composites

XU Dongwei¹^,², WANG Ruiqi¹, CHEN Ping¹(

)

1 State Key Laboratory of Fine Chemicals, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, China
2 School of Material Science and Engineering, Zhengzhou University of Aeronautics, Zhengzhou 450046, China

引用本文:

徐东卫, 王瑞琪, 陈平. 石墨烯基吸波复合材料研究进展[J]. 材料研究学报, 2024, 38(1): 1-13.
Dongwei XU, Ruiqi WANG, Ping CHEN. Research Progress of Graphene-based Absorbing Composites[J]. Chinese Journal of Materials Research, 2024, 38(1): 1-13.

全文: PDF(14834 KB) HTML

摘要:

电子信息技术的迅速发展，致使电磁污染及干扰问题愈加严重，研制具有“宽、薄、轻、强”综合优异性能的吸波材料显得尤为重要。石墨烯材料因其具有轻质、高导电、大比表面积、强介电损耗等优点，但其阻抗匹配性能较差，损耗机制单一。对其进行异质元素掺杂或进行形貌结构设计，可有效改善其阻抗失配问题。本文基于电磁波吸收理论，阐述了不同维度石墨烯基吸波复合材料的研究进展，详细讨论了不同石墨烯基吸波复合材料的性能和吸波机理。还讨论了石墨烯吸波材料领域目前研究工作中存在的一些不足，最后针对石墨烯基吸波材料未来的研究方向和发展前景进行了展望。

关键词 ：评述, 石墨烯, 微波吸收, 结构调控, 多功能吸波材料, 阻抗匹配

Abstract：

With the rapid development of electronic information technology, electromagnetic pollution and interference have become more and more serious. It is particularly important to develop microwave absorption materials with comprehensive excellent performance of "wide, thin, light and strong". Graphene materials have the advantages of light weight, high conductivity, large specific surface area and strong dielectric loss, however, the impedance matching performance is poor and the loss mechanism is single. Interestingly, the impedance mismatch can be effectively improved by doping heterogeneous elements or designing morphology and structure. Herein, based on electromagnetic wave absorption theory, this paper describes the research progress of different dimensions of graphene-based absorbing materials, and discusses the properties and microwave absorbing mechanism of different graphene-based absorbing materials in detail. The shortcomings of current research work in the field of graphene absorbing materials are also discussed. Finally, the future research direction and development prospect of graphene-based absorbing materials are prospected.

Key words： review graphene microwave absorption texture regulation multifunctional absorbing material impedance matching

收稿日期: 2023-02-04

ZTFLH:

TB332

基金资助:国家重大研究计划(2019-ZD-380-12);兴辽英才计划(XLYC1802085);大连市科技创新基金重大项目(2019J11CY007);中央高校基本科研基金(DUT18GF107);航空科学基金(20173754009);河南省自然科学基金(232300420332);河南省高等学校重点科研项目(23A430006)

通讯作者: 陈平，教授，pchen@dlut.edu.cn，研究方向为高性能高分子材料与先进聚合物基复合材料结构与功能一体化设计与制备

Corresponding author: CHEN Ping, Tel: (0411)84986100, E-mail: pchen@dlut.edu.cn

作者简介: 徐东卫，男，1990年生，博士

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图1 电磁波的传输及和吸波材料作用的示意图

图2 三种类型吸波性能测量技术示意图[21]

图3 疏水Fe3O4-石墨烯杂化物的制备流程示意图[24]

图4 CoS2/rGO纳米杂化物的结构和性能[31]

图5 Air@rGO€Fe3O4空心微球的制备示意图[33]

图6 空心氧化石墨烯气凝胶微球和球中球氧化石墨烯气凝胶微球的示意图[36]

图7 f-GO、f-GO纤维和还原f-GO纤维的制备示意图[42]

图8 皮芯型石墨烯/MXene纤维气凝胶的制备及其应用[44]

图9 三维“泡沫型”结构石墨烯的电磁波损耗模型及其典型性能对比[49]

图10 3D磁性石墨烯泡沫复合材料的制备工艺流程[50]

图11 CNT/RGO/CoNi链杂化气凝胶制备工艺示意图[56]

图12 复合气凝胶开/关微波吸收模式示意图[61]

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