Research Progress on Stability of CsPbI2Br Inorganic Perovskite Solar Cells

doi:10.11901/1005.3093.2020.158

Chinese Journal of Materials Research

2020, Vol. 34

Issue (11): 811-821 DOI: 10.11901/1005.3093.2020.158

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Research Progress on Stability of CsPbI₂Br Inorganic Perovskite Solar Cells

WU Qiaofeng¹, ZHANG Fu¹, YU Yue¹, ZHANG Meng¹, YU Hua¹(

), FAN Shuanshi²(

)

^1.Institute of Photovoltaics, Southwest Petroleum University, Chengdu 610500, China
^2.Key Laboratory of Heat Transfer Enhancement and Energy Conservation of Education Ministry, South China University of Technology, Guangzhou 510640, China

Cite this article:

WU Qiaofeng, ZHANG Fu, YU Yue, ZHANG Meng, YU Hua, FAN Shuanshi. Research Progress on Stability of CsPbI₂Br Inorganic Perovskite Solar Cells. Chinese Journal of Materials Research, 2020, 34(11): 811-821.

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Abstract

Inorganic perovskite materials have excellent thermal stability due to that the volatile organic components (MA⁺, FA⁺) in organic-inorganic hybrid perovskite materials are completely replaced by cesium ions (Cs⁺). Inorganic perovskite solar cells (IPSCs) are favored by researchers internationally due to their excellent thermal stability. Since the CsPbI₂Br was used as the photoactive layer for the first time in 2016, its photoelectric conversion efficiency (PCE) increased from 9.84% to 18.06%, but the device stability of IPSCs still restricts its commercial application progress. This paper reviews the unstable factors of CsPbI₂Br IPSCs and summarizes the recent research progress on the stability of CsPbI₂Br IPSCs from three aspects: preparation methods, ion doping, and interface optimization. Finally, an outlook on the research challenges and prospects of CsPbI₂Br based IPSCs was proposed and discussed.

Key words: review inorganic nonmetallic materials inorganic perovskite solar cells stability CsPbI₂Br

Received: 11 May 2020

ZTFLH:

TM 914.4

Fund: Scientific Research Starting the Project of SWPU(X151528)

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	Qiaofeng WU
	Fu ZHANG
	Yue YU
	Meng ZHANG
	Hua YU
	Shuanshi FAN

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https://www.cjmr.org/EN/10.11901/1005.3093.2020.158 OR https://www.cjmr.org/EN/Y2020/V34/I11/811

Fig.1 Evolution of CsPbI₂Br perovskite solar cell energy conversion efficiencies

Fig.2 Mechanism of the moisture-triggered phase transition in inorganic perovskites (a) the moisture induce perovskite to form vacancies, (b) vacancies enter the lattice and cause perovskite to triggered phase transition^[22]

Fig.3 Molecular structure and properties of solvents commonly used in perovskite precursors^[47] (a), schematic of the evolution of the CsPbI₂Br film with the introduction of DMSO^[48] (b), SEM images of CsPbI₂Br films annealed at the temperature range from 100 to 350℃ for 2 min. Scale bar: 1 μm^[57] (c) and schematic illustration of CsPbI₂Br perovskite crystallization process via GTA or GTA-ATS processing^[58] (d)

Fig.4 Schematic diagram of a typical three-dimensional perovskite crystal structure^[65] (a), SEM images of undoped CsPbI₂Br (A) and CsPb_0.95Eu_0.05I₂Br perovskite films (B)^[78] (b) and schematic diagram of device structure and two modes of Mn^{2 +} doped in the gap and replacing Pb^2+[80] (c)

Fig.5 Schematic architecture of CsPbI₂Br planar IPSCs inserted into MoO₃ interface layer^[89] (a), SEM images of a) CsPbI₂Br/BT1, b) CsPbI₂Br/BT2 and c) CsPbI₂Br/BT3 films^[90] (b) and process of synthesis 2D/3D perovskite by SIM method^[26] (c)

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