Research Progress of MXene Used in Lithium Sulfur Battery

doi:10.11901/1005.3093.2022.360

Chinese Journal of Materials Research

2023, Vol. 37

Issue (7): 481-494 DOI: 10.11901/1005.3093.2022.360

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Research Progress of MXene Used in Lithium Sulfur Battery

JI Yuchen, LIU Shuhe(

), ZHANG Tianyu, ZHA Cheng

Faculty of Metallurgy and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China

Cite this article:

JI Yuchen, LIU Shuhe, ZHANG Tianyu, ZHA Cheng. Research Progress of MXene Used in Lithium Sulfur Battery. Chinese Journal of Materials Research, 2023, 37(7): 481-494.

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Abstract

As an emerging two-dimensional transition metal carbide or carbonitride, MXene exhibits excellent metallic conductivity, abundant surface functional groups and ultrathin two-dimensional structure, which endows it great potential in electrochemical energy storage. Lithium-sulfur batteries have a high theoretical specific capacity and become a very competitive choice in the new generation of energy storage devices. Two-dimensional MXenes and the assembled three-dimensional materials, as advanced sulfur carriers, can effectively improve the inherent poor conductivity and serious dissolution of discharge products of lithium-sulfur batteries. This paper reviews the current applications of MXene materials with two-dimensional and three-dimensional structures in lithium-sulfur batteries, analyzes the relationship between different structures and performance, summarizes the current challenges and difficulties, and gives a view on the direction to proceed for future designs.

Key words: review MXene lithium sulfur battery composites

Received: 01 July 2022

ZTFLH:

O646

Fund: National Natural Science Foundation of China(51264016)

Corresponding Authors: LIU Shuhe, Tel: 15912595890, E-mail: 2538234121@qq.com

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	JI Yuchen
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	ZHANG Tianyu
	ZHA Cheng

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https://www.cjmr.org/EN/10.11901/1005.3093.2022.360 OR https://www.cjmr.org/EN/Y2023/V37/I7/481

Fig.1 Electrochemical reaction schematic diagram (a) and charge-discharge profile (b) of lithium-sulfur battery^[7,10]

Fig.2 Diagram of "shuttle effect"^[19]

Fig.3 SEM images of MXene before (a) and after (b) eatching^[31]

Fig.4 Structural formation diagram of MXene^[35]

Fig.5 Synthesis schematic of the crumpled N-Ti₃C₂T _x /S nanosheets^[37]

Fig.6 Schematic diagram of the in-situ sulfidation by thiourea^[45]

Fig.7 Schematic diagram of CTF/TNS heterostructure^[46]

Fig.8 SEM image of MXene@TiO₂ nanoarrays^[47]

Fig.9 FESEM images of CoZn-MOFs@MX^[38]

Fig.10 Synthesis schematic and SEM image of MXene/RGO nanosheets^[52]

Fig.11 SEM and HRTEM images of MXene/MoS₂-C nanocomposite^[53]

Fig.12 Schematic diagram of the synthesis process of (sulfur-impregnated) Co-MoSe₂/MXene^[54]

Fig.13 Schematic diagrams of Ti₃C₂T _x @AlF₃ and layered Ti₃C₂T _x @AlF₃/NH composites^[56]

Fig.14 Schematic diagram of the structure of dTCP and cross-sectional SEM image

Fig.15 Schematic of synthesizing PA-MXene/CNT with unidirectional freeze-drying process^[58]

Fig.16 (a) Schematic diagram of the “three regions” and (b) cycling performance of the cathode at 0.05C for sulfur loading of 10 mg·cm^-2[59]

Fig.17 Structural schematic and SEM images of Ti₃C₂T _x -CNT composites^[62]

Fig.18 Schematic illustration of the MF-templating synthesis of P-NTC composites^[63]

Fig.19 SEM and EDS images of hollow Co-CNT@MXene^[65]

Fig.20 SEM images of S-CNT and S-CNT@MXene spheres^[66]

Fig.21 Synthesis schematic and cross-section SEM images of S@PCL

Fig.22 Synthesis schematic and SEM images of N‑Ti₃C₂@CNT composites^[68]

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