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材料研究学报  2026, Vol. 40 Issue (9): 697-709    DOI: 10.11901/1005.3093.2025.354
  研究论文 本期目录 | 过刊浏览 |
高氯煤烟中的氯腐蚀锅炉换热器的机理
郭非凡1, 马继刚1, 陈丽娟1,2(), 谢伟智1, 魏博1,2(), 马瑞3, 安田田1, 李奕华1, 李新月1
1.新疆大学化工学院 乌鲁木齐 830017
2.新疆煤炭清洁转化与化工过程重点实验室 乌鲁木齐 830017
3.新疆大学电气工程学院 乌鲁木齐 830017
Corrosion Behavior of 12Cr1MoVG Steel in a Simulated Flue Gas for High-chlorine Coal while Containing Different Forms of Chlorine
GUO Feifan1, MA Jigang1, CHEN Lijuan1,2(), XIE Weizhi1, WEI Bo1,2(), MA Rui3, AN Tiantian1, LI Yihua1, LI Xinyue1
1.School of Chemical Engineering, Xinjiang University, Urumqi 830017, China
2.Xinjiang Key Laboratory of Clean Coal Conversion and Chemical Processes, Urumqi 830017, China
3.School of Electrical Engineering, Xinjiang University, Urumqi 830017, China
引用本文:

郭非凡, 马继刚, 陈丽娟, 谢伟智, 魏博, 马瑞, 安田田, 李奕华, 李新月. 高氯煤烟中的氯腐蚀锅炉换热器的机理[J]. 材料研究学报, 2026, 40(9): 697-709.
Feifan GUO, Jigang MA, Lijuan CHEN, Weizhi XIE, Bo WEI, Rui MA, Tiantian AN, Yihua LI, Xinyue LI. Corrosion Behavior of 12Cr1MoVG Steel in a Simulated Flue Gas for High-chlorine Coal while Containing Different Forms of Chlorine[J]. Chinese Journal of Materials Research, 2026, 40(9): 697-709.

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摘要: 

模拟高氯煤烟气(Cl2/HCl + CO2 + H2O + N2,550 ℃/650 ℃)的多组分可控气氛,进行了其对锅炉换热器12Cr1MoVG钢的高温腐蚀实验,根据腐蚀产生的质量损失、SEM-EDS、XRD谱和热力学计算结果研究了腐蚀的机理。结果表明温度对12Cr1MoVG钢腐蚀的影响较大。温度从550 ℃提高到650 ℃,这种钢表面氧化膜的厚度增加了232.4 µm,腐蚀产生的质量损失增加了21.26 mg/cm2,钢的表面氧化膜产生了微裂纹等缺陷。在相同的条件下,Cl2对12Cr1MoVG钢的腐蚀比HCl严重。这种钢的试样被HCl腐蚀后表面生成易挥发的FeCl2,FeCl2挥发产生的孔隙使HCl穿过氧化膜与金属基底发生反应,使氧化膜产生横向和纵向裂纹;而试样被Cl2腐蚀后表面生成的FeCl3在更低的温度挥发后产生密集的孔洞,Cl2通过孔洞向内渗透与基底反应使表面的氧化膜严重分层和脱落。Cl2对锅炉换热器12Cr1MoVG钢的高温腐蚀是一种自催化循环过程:HCl、Cl2与钢反应生成易挥发的铁基氯化物(FeCl2、FeCl3),这种铁基氯化物挥发后与H2O发生氧化反应生成HCl,于是形成循环腐蚀最终使氧化膜分层脱落。Cl2的氧化性更强,生成的易挥发腐蚀产物比HCl更多。

关键词 : 金属材料,  高温腐蚀,  氯腐蚀,  高氯煤燃烧,  12Cr1MoVG    
Abstract:

The flue gas generated from combustion of high-chlorine containing coals may induce severe corrosion on boiler heat exchanger tubes due to chlorine-containing species, significantly compromising the operational safety. Herein the high-temperature corrosion behavior of boiler steel 12Cr1MoVG was investigated in flue gas containing different chlorine species. For this purpose, a high-temperature corrosion test rig was established to simulate the flue gas environment (Cl2/HCl + CO2 + H2O + N2, 550 oC/650 oC) in boilers firing high-chlorine coal while containing different forms of chlorine. The corrosion behavior of the steel was characterized by means of mass loss measurement, SEM-EDS, XRD, and thermodynamic calculations. The results revealed that temperature significantly influences material corrosion. When temperature increased from 550 oC to 650 oC, oxide scale thickness increased by 232.4 µm with a corresponding mass loss increase of 21.26 mg/cm2. Microcracks developed in the surface oxide scale due to thermal stress. Under identical conditions, Cl2 induced more severe corrosion than HCl. When the corrosion of steel in artificial flue gas containing HCl may generate volatile FeCl2, whose sublimation created porous pathways allowing HCl penetration through the oxide scale to react with the steel substrate, simultaneously inducing transverse and longitudinal cracks. In contrast, when exposure to ones containing Cl2 the steel corrosion could induce the formation of FeCl3, which volatilizes at lower temperatures, producing dense porosity that facilitated inward chlorine diffusion and subsequent reaction with the steel substrate, ultimately causing severe oxide scale delamination and spallation. Chlorine-induced high-temperature corrosion of the steel follows an autocatalytic cycle: HCl/Cl2 reacts with the steel to form volatile iron chlorides (FeCl2/FeCl3). These compounds volatilize and undergo oxidation with H2O, regenerating HCl to sustain the corrosive cycle. This process ultimately leads to metallic oxide scale degradation through delamination and spallation. The stronger oxidizing capability of Cl2 and higher volatility of its corrosion products result in more severe material degradation compared to HCl.

Key words: metallic materials    high-temperature corrosion    chlorine corrosion    high-chlorine coal combustion    12Cr1MoVG
收稿日期: 2025-11-27     
ZTFLH:  TG172  
基金资助:高校青年教师科研创新能力支持项目(SRICSPYF-BS2025042);国家自然科学基金(52261022);2025年国家级大学生创新训练计划项目(202510755044)
通讯作者: 陈丽娟,副教授,ljchenxju@163.com,研究方向为过程装备结构优化,金属材料腐蚀与防护;
魏博,教授,weiboxju@163.com,研究方向为固体颗粒物燃烧与燃烧污染物控制
Corresponding author: CHEN Lijuan, Tel: 18016827217, E-mail: ljchenxju@163.com;
WEI Bo, Tel: 18703028892, E-mail: weiboxju@163.com
作者简介: 郭非凡,男,2001年生,硕士生
Alloy steelFePCrSiMnSCCuMoV
12Cr1MoVG97.670.0090.980.280.470.0020.120.080.280.17
表1  12Cr1MoVG钢的化学成分
图1  可控气氛高温腐蚀实验台的示意图
GroupCO2H2OHClCl2N2T / oCTotal flow
N218%10%//Bal.

550

650

250 mL/min
HCl18%10%0.05%/
Cl218%10%/0.05%
表2  气体的组成和实验工况
图2  12Cr1MoVG钢在550 ℃、650 ℃的N2、HCl、Cl2气氛中腐蚀100 h后的质量损失
图3  12Cr1MoVG钢在N2、HCl、Cl2气氛中不同温度腐蚀20 h和100 h后的宏观形貌
图4  12Cr1MoVG钢在N2、HCl、Cl2气氛中不同温度腐蚀100 h后的微观形貌
图5  12Cr1MoVG钢试样在N2、HCl、Cl2气氛中不同温度腐蚀100 h表面的XRD谱
图6  12Cr1MoVG钢试样在550 ℃腐蚀100 h后截面的元素分布
图7  12Cr1MoVG钢试样在650 ℃腐蚀100 h后截面的元素分布
图8  12Cr1MoVG钢试样在550 ℃腐蚀100 h后截面的线扫描图
图9  12Cr1MoVG钢试样在650 ℃下腐蚀100 h后截面的线扫描图
图10  Fe、Cr、Mn和V与H2O、HCl、Cl2及MCl x 与H2O在450 ℃~750 ℃反应的热力学参数
Metal chloridesMelting point / oCSaturated vapor pressure / Pa
550 oC650 oC
FeCl26762 × 1015 × 102
FeCl33031.5 × 1048 × 104
CrCl28201 × 10-35 × 10-2
CrCl311501.5 × 1015 × 102
MnCl26503 × 1008 × 101
VCl310278 × 1004.5 × 101
表3  铁、铬、锰氯化物的熔点和饱和蒸气压
图11  12Cr1MoVG钢在HCl (a)、Cl2 (b)中的高温腐蚀机理
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