Preparation of Y2O3 Hollow Spheres and Low Frequency Damping Properties of Rubber Composite Reinforced with Y2O3 Hollow Spheres

doi:10.11901/1005.3093.2014.536

Chinese Journal of Materials Research

2015, Vol. 29

Issue (7): 505-510 DOI: 10.11901/1005.3093.2014.536

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Preparation of Y₂O₃Hollow Spheres and Low Frequency Damping Properties of Rubber Composite Reinforced with Y₂O₃Hollow Spheres

Fuqing ZHANG¹,Wei WANG²,Gang SUN²,Jiangtao CHEN²,Xueliang JIANG^2,^**(

)

1. School of Chemical and Environmental Engineering, Wuhan Institute of Technology, Wuhan 430073, China
2. School of Material Science and Engineering, Wuhan Institute of Technology, Wuhan 430073, China

Cite this article:

Fuqing ZHANG,Wei WANG,Gang SUN,Jiangtao CHEN,Xueliang JIANG. Preparation of Y₂O₃Hollow Spheres and Low Frequency Damping Properties of Rubber Composite Reinforced with Y₂O₃Hollow Spheres. Chinese Journal of Materials Research, 2015, 29(7): 505-510.

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Abstract

Poly(methyl methacrylate) (PMMA) spheres were firstly prepared through dispersion polymerization, then with which as sacrifice template, PMMA/Y(OH)CO₃ composite microspheres were prepared by homogeneous precipitation technique. Thirdly, Y₂O₃ hollow spheres were obtained by calcination of PMMA/Y(OH)CO₃at elevated temperature, and finally Y₂O₃ hollow shperes reinforced butyl rubber composites were fabricated. The structure and morphology of the Y₂O₃ hollow nanospheres were characterized by means of Fourier transform infrared spectroscopy (FTIR), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray photoelectron spectrum (XPS), X-ray diffraction (XRD) and thermogravimetry (TG). The results show that hollow spheres composed of Y₂O₃particles of face-centered cubic crystallorgraphic structure, and their diameter is about 1 μm with a thin shell thickness about 80 nm. The hollow microspheres and powders of Y₂O₃ as filler were added respectively into butyl rubber to prepare butyl rubber composites. It follows that the butyl rubber composites with addition of Y₂O₃ hollow spheres rather than that of Y₂O₃ powders exhibited better damping properties with larger loss factors by frequencies such as 8, 18, 28, 50, 65 and 90 Hz.

Key words: composites polymethyl methacrylate template Y₂O₃ hollow nanospheres low frequency damping capacity butyl rubber

Received: 26 September 2014

Fund: *Supported by National Natural Science Foundation of China No. 51273154, Graduate Education Innovation project Wuhan Institute of Technology CX2013085, and Open Foundation of Key Laboratory for Green Chemical Process of Ministry of Education No. GCP201307.

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	Fuqing ZHANG
	Wei WANG
	Gang SUN
	Jiangtao CHEN
	Xueliang JIANG

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https://www.cjmr.org/EN/10.11901/1005.3093.2014.536 OR https://www.cjmr.org/EN/Y2015/V29/I7/505

Fig.1 SEM image of PMMA spheres (a), PMMA/Y(OH)CO₃ composite spheres (b), Y₂O₃ hollow spheres (c) and TEM image of Y₂O₃ hollow spheres (d)

Fig.2 FT-IR spectrum of PMMA spheres (a), PMMA/Y(OH)CO₃ composite spheres (b) and Y₂O₃ hollow spheres (c)

Fig.3 TG curves of PMMA spheres (a), PMMA/Y(OH)CO₃ composite spheres (b) and Y₂O₃ hollow spheres (c)

Fig.4 XRD patterns of Y₂O₃hollow spheres calcined at 500℃ (a), 700℃ (b) and 900℃ (c)

Fig.5 XPS wide spectrum (a) and Y 3d spectrum (b) of Y₂O₃ hollow nanospheres

Fig.6 Damping capacity of composites in different temperature (frequency 1 Hz) (a) IIR/Y₂O₃ hollow sphere = 100/30, (b) IIR/Y₂O₃ power = 100/30, (c) IIR

Fig.7 The damping capacity of composites at different frequency (a) IIR/Y₂O₃ hollow sphere = 100/30, (b) IIR/Y₂O₃ power = 100/30

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