Damping Enhancement of Graphene/Polymer Composites Based on Interfacial Interactions of Hydrogen Bonds

doi:10.11901/1005.3093.2022.337

Chinese Journal of Materials Research

2023, Vol. 37

Issue (6): 401-407 DOI: 10.11901/1005.3093.2022.337

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Damping Enhancement of Graphene/Polymer Composites Based on Interfacial Interactions of Hydrogen Bonds

ZHANG Tengxin¹^,², WANG Han¹(

), HAO Yabin¹^,², ZHANG Jiangang¹^,², SUN Xinyang¹^,², ZENG You¹^,²(

)

^1.Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, China
^2.School of Materials Science and Engineering, University of Science and Technology of China, Shenyang 110016, China

Cite this article:

ZHANG Tengxin, WANG Han, HAO Yabin, ZHANG Jiangang, SUN Xinyang, ZENG You. Damping Enhancement of Graphene/Polymer Composites Based on Interfacial Interactions of Hydrogen Bonds. Chinese Journal of Materials Research, 2023, 37(6): 401-407.

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Abstract

Developing advanced composites with high strength and high vibration damping is extremely important for ensuring high safety and reliability of composites in high-frequency-vibration circumstances. In this paper, we proposed a novel strategy to remarkably enhance the damping property of composites by introducing reversible hydrogen bonds at the interfaces of graphene/polymer composites. Graphene and poly(styrene-ethylene-butadiene-styrene) (SEBS) were chemically modified to graft hydrogen bonding moiety, consequently forming multiple hydrogen-bonding networks at interfaces of graphene/SEBS composites. The cyclic tensile behavior and dynamic mechanical properties of the composites were investigated in detail. The results showed that the mechanical and damping properties of graphene/SEBS composites were greatly improved by introducing graphene and interfacial hydrogen-bonding structures. The elastic modulus, hysteresis loss, and damping ratio of the graphene/SEBS composites were increased by 165%, 237% and 42% in comparison with that of SEBS. Such remarkable enhancement in both mechanical and damping properties is mainly attributed to the interfacial hydrogen bonds between components, high-efficiency stress-transferring, and significant energy dissipation resulted from reversible breaking/formation of hydrogen bonds during cyclic deformation.

Key words: composites damping properties interfacial hydrogen bonds graphene mechanical strength

Received: 20 June 2022

ZTFLH:

TB332

Fund: National Natural Science Foundation of China(52130209);National Natural Science Foundation of China(51802317);Liaoning Natural Science Foundation(2019JH3/30100008);Opening Foundation of Shanxi Key Laboratory of Nano & Functional Composite Materials(NFCM202102);IMR Innovation Fund(2022-PY07);Shenyang National Laboratory for Materials Science(2021-FP31)

Corresponding Authors: ZENG You, Tel:(024)83978090, E-mail: yzeng@imr.ac.cn;
WANG Han, Tel:(024)83978090, E-mail: hanwang@imr.ac.cn

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	ZHANG Tengxin
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	ZENG You

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https://www.cjmr.org/EN/10.11901/1005.3093.2022.337 OR https://www.cjmr.org/EN/Y2023/V37/I6/401

Fig.1 Schematics of interfacial hydrogen bonds in Gr/SEBS composites (a) ATA-grafted SEBS, (b) ATA-modified graphene, and (c) the interfacial hydrogen bonds between components

Fig.2 Infrared spectra of the GO, m-Gr, SEBS, m-SEBS, and Gr/SEBS composites (a) and In-situ infrared spectra (b) of Gr/SEBS composites at variable temperatures

Fig.3 Cyclic tensile mechanical behavior of Gr/SEBS composites (a) cyclic tensile stress-strain curve, (b) tensile modulus, (c) tensile stress at 400% strain, and (d) hysteresis loss

Fig.4 Dynamic mechanical analyses of Gr/SEBS composites (a) storage modulus, (b) loss modulus, (c) tanδ, and (d) the storage modulus and damping ratio against graphene loadings

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